This paper described how university students from Macau took social responsibility in China through Service-Learning project. It was an introductory experience for the student participants and for the children in the mountain area as well. This study aimed at raising children's interest in learning and their desire of continuing study. Results were reported in four themes: (1) increasing personal competence of teamwork spirits, leadership and service skills; (2) students' perception towards poverty issue and education in China rural and mountain areas; (3) having commitment to the next service; (4) realizing that Service-Learning must be a mutual process. This paper also provides an overview of how a living-learning community dedicated itself to community service to educate residents holistically.