This article delineates the foundational theological principles upon which a Catholic Higher Education chaplaincy devoted to the spiritual development of staff and students might rest. We claim that this is a key dimension of chaplaincy work. In a (post)modern culture where staff and students exhibit a range of beliefs or none, we offer a broad definition of spirituality not necessarily tied to religion and construct a framework which might appeal to a wide cross section of people attending Catholic Universities. It examines how the insights and guidance of two French Catholic writers, the 16th century priest St. Francis de Sales and the contemporary philosopher Jean-Luc Marion, offer a basis for understanding what constitutes a spiritual approach to life. We suggest that their emphases on the power of love, the heart, God's glory, "imago Dei" and gift constitute a ground of hope and stable base from which spiritual progress might take place. We also outline how this template challenges the emphasis on autonomous agency at the centre of much educational discourse at the present time.